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1.
F. C. Fehsenfeld M. J. Bollinger S. C. Liu D. D. Parrish M. McFarland M. Trainer D. Kley P. C. Murphy D. L. Albritton D. H. Lenschow 《Journal of Atmospheric Chemistry》1983,1(1):87-105
The seasonal and diurnal variations of ozone mixing ratios have been observed at Niwot Ridge. Colorado. The ozone mixing ratios have been correlated with the NO
x
(NO+NO2) mixing ratios measured concurrently at the site. The seasonal and diurnal variations in O3 can be reasonably well understood by considering photochemistry and transport. In the winter there is no apparent systematic diurnal variation in the O3 mixing ratio because there is little diurnal change of transport and a slow photochemistry. In the summer, the O3 levels at the site are suppressed at night due to the presence of a nocturnal inversion layer that isolated ozone near the surface, where it is destroyed. Ozone is observed to increase in the summer during the day. The increases in ozone correlate with increasing NO
x
levels, as well as with the levels of other compounds of anthropogenic origin. We interpret this correlation as in-situ or in-transit photochemical production of ozone from these precursors that are transported to our site. The levels of ozone recorded approach 100 ppbv at NO
x
mixing ratios of approximately 3 ppbv. Calculations made using a simple clean tropospheric chemical model are consistent with the NO
x
-related trend observed for the daytime ozone mixing ratio. However, the chemistry, which does not include nonmethane hydrocarbon photochemistry, underestimates the observed O3 production. 相似文献
2.
Effects of Mesoscale Surface Thermal Heterogeneity on Low-Level Horizontal Wind Speeds 总被引：2，自引：2，他引：0
Using large-eddy simulation, we investigate characteristics of horizontal wind speed at 100 m above the ground, with surface
heat-flux variations that are sinusoidal with amplitudes of 0, 50, and 200 W m−2 and wavelengths of 16, 32, and 128 km, and no background flow. When the amplitude is 200 W m−2, wind speeds induced by the surface-flux variations on scales of 16 and/or 32 km have multiple temporal oscillations from
0600 to 1800 local standard time. The positive peaks first appear before noon. In contrast, for wind speeds induced by the
128-km surface heterogeneity, a single oscillation occurs in the late afternoon, which is much larger than those generated
by the 16- and 32-km surface heterogeneity. In addition, at the oscillation onset the kurtosis of the velocity increment over
a distance of 1 km significantly increases, which implies intermittency in the generation of 1-km scale eddies. The spatially
intermittent energy cascade generated by surface heterogeneity scaled down to 1-km eddies is analogous to the well-known intermittent
energy cascade in the inertial subrange. The kurtosis of the 1-km eddies is much larger with the 128-km surface heterogeneity
than with the 16- and 32-km heterogeneities. Thus we conclude that localized rapid changes of low-level horizontal wind speed
may be caused by significant local surface heterogeneity on scales between a few tens and a few hundreds of kilometres. 相似文献
3.
An Improved Approach for Parameterizing Surface-Layer Turbulent Transfer Coefficients in Numerical Models 总被引：2，自引：0，他引：2
Based on classic iterative computation results, new equations to calculate the surface turbulent transfer coefficients are
proposed, which allow for large ratios of the momentum and heat roughness lengths. Compared to the Launiainen scheme, our
proposed scheme generates results closer to classical iterative computations. Under unstable stratification, the relative
error in the Launiainen scheme increases linearly with increasing instability, even exceeding 15%, while the relative error
of the present scheme is always less than 8.5%. Under stable stratification, the Launiainen scheme uses two equations, one
for 0 < Ri
B ≤ 0.08 and another for 0.08 < Ri
B ≤ 0.2, and does not consider the condition that Ri
B > 0.2, while its relative errors in the region 0 < Ri
B ≤ 0.2 exceed 31 and 24% for momentum and heat transfer coefficients, respectively. In contrast, the present scheme uses only
one equation for 0 < Ri
B ≤ 0.2 and another equation for Ri
B > 0.2, and the relative error of the present scheme is always less than 14%. 相似文献
4.
Doppler Lidar Measurements of Vertical Velocity Spectra in the Convective Planetary Boundary Layer 总被引：1，自引：1，他引：0
We utilized a Doppler lidar to measure spectra of vertical velocity w from 390m above the surface to the top of the daytime convective boundary layer (CBL). The high resolution 2μm wavelength
Doppler lidar developed by the NOAA Environmental Technology Laboratory was used to detect the mean radial velocity of aerosol
particles. It operated continuously during the daytime in the zenith-pointing mode for several days in summer 1996 during
the Lidars-in-Flat-Terrain experiment over level farmland in central Illinois, U.S.A. The temporal resolution of the lidar
was about 1 s, and the range-gate resolution was about 30m. The vertical cross-sections were used to calculate spectra as
a function of height with unprecedented vertical resolution throughout much of the CBL, and, in general, we find continuity
of the spectral peaks throughout the depth of the CBL. We compare the observed spectra with previous formulations based on
both measurements and numerical simulations, and discuss the considerable differences, both on an averaged and a case-by-case
basis. We fit the observed spectra to a model that takes into account the wavelength of the spectral peak and the curvature
of the spectra across the transition from low wavenumbers to the inertial subrange. The curvature generally is as large or
larger than the von Kármán spectra. There is large case-to-case variability, some of which can be linked to the mean structure
of the CBL, especially the mean wind and the convective instability. We also find a large case-to-case variability in our
estimates of normalized turbulent kinetic energy dissipation deduced from the spectra, likely due for the most part to a varying
ratio of entrainment flux to surface flux. Finally, we find a relatively larger contribution to the low wavenumber region
of the spectra in cases with smaller shear across the capping inversion, and suggest that this may be due partly to gravity
waves in the inversion and overlying free atmosphere. 相似文献
5.
A set of new parameterizations for the friction velocity and temperature scale over gently
sloped terrain and in calm synoptic conditions are theoretically derived. The friction velocity is
found to be proportional to the product of the square root of the total accumulated heating in the
boundary layer and the sinusoidal function of the slope angle, while the temperature scale is
proportional to the product of the boundary layer depth, the sinusoidal function of the slope angle
and the potential temperature gradient in the free atmosphere. Using the new friction velocity
parameterization, together with a parameterization of eddy diffusivity and an initial potential
temperature profile around sunrise, an improved parameterization for the thermally induced upslope
flow profile is derived by solving the Prandtl equations. The upslope flow profile is found to be
simply proportional to the friction velocity. 相似文献
6.
河北承德黑山铁矿床热液成矿特征及流体包裹体研究 总被引：3，自引：2，他引：1
黑山大型钒钛磁铁矿矿床产于大庙斜长岩杂岩体中,是承德地区最重要的"大庙式"岩浆型铁矿床。笔者在矿区野外地质观察过程中发现,穿插于斜长岩中的铁磷矿脉、磁铁矿硫化物矿脉有热液成矿作用的显示,表明黑山铁矿床成因除传统认为的岩浆期结晶、熔离、矿浆贯入成矿作用外,还有热液期的成矿作用发生。本文对热液成矿期铁磷矿石中磷灰石和矿化蚀变石英中的流体包裹体进行了显微测温和激光拉曼光谱分析。结果表明,磷灰石中原生包裹体可以分为气液两相包裹体、含子矿物包裹体、含液态CO2三相包裹体、单液相、单气相包裹体5类,均一温度主要集中于180～420℃,盐度主要集中于6.2%～38.9%NaCleq,流体包裹体气相成分主要为CO2、N2和CH4,液相成分主要为H2O,固相成分主要为方解石、石盐、白云石及铁氧化物子矿物。石英中流体包裹体类型和成分与磷灰石中的类似,但固相成分未发现石盐和不透明金属子矿物,均一温度变化于149～422℃,盐度变化于5.7%～22.9%NaCleq。成矿流体为CaCl2-NaCl-H2O-CO2体系,均一温度和盐度呈现正相关连续渐变的特征。铁磷矿石的磷灰石中原生包裹体为流体包裹体,盐度高,子矿物种类复杂,组成中富含CO2和CH4等,这些特征显示成矿流体以岩浆热液为主;成矿机理可能与大气降水对岩浆热液的稀释有关。 相似文献
7.
Jielun Sun Donald H. Lenschow Sean P. Burns Robert M. Banta Rob K. Newsom Richard Coulter Stephen Frasier Turker Ince Carmen Nappo Ben B. Balsley Michael Jensen Larry Mahrt David Miller Brian Skelly 《Boundary-Layer Meteorology》2004,110(2):255-279
Using the unprecedented observational facilities deployed duringthe 1999 Cooperative Atmosphere-Surface Exchange Study (CASES-99),we found three distinct turbulent events on the night of 18October 1999. These events resulted from a density current,solitary wave, and internal gravity wave, respectively. Our studyfocuses on the turbulence intermittency generated by the solitarywave and internal gravity wave, and intermittent turbulenceepisodes associated with pressure change and wind direction shiftsadjacent to the ground. Both the solitary and internal gravitywaves propagated horizontally and downward. During the passage ofboth the solitary and internal gravity waves, local thermal andshear instabilities were generated as cold air was pushed abovewarm air and wind gusts reached to the ground. These thermal andshear instabilities triggered turbulent mixing events. Inaddition, strong vertical acceleration associated with thesolitary wave led to large non-hydrostatic pressure perturbationsthat were positively correlated with temperature. The directionaldifference between the propagation of the internal gravity waveand the ambient flow led to lateral rolls. These episodic studiesdemonstrate that non-local disturbances are responsible for localthermal and shear instabilities, leading to intermittentturbulence in nocturnal boundary layers. The origin of thesenon-local disturbances needs to be understood to improve mesoscalenumerical model performance. 相似文献
8.
L. Kristensen D. H. Lenschow P. Kirkegaard M. Courtney 《Boundary-Layer Meteorology》1989,47(1-4):149-193
We have postulated a simple model for the spectral tensor
ij
(k) of an anisotropic, but homogeneous turbulent velocity field. It is a simple generalization of the spectral tensor
inf
ij
piso(k) for isotropic turbulence and we show how in the limit of isotropy,
ij
(k) becomes equal to
inf
ij
piso(k). Whereas
inf
ij
piso(k) is determined entirely by one scalar function of k = ¦k¦, namely the energy spectrum, we need three independent scalar functions of k to specify
ij
(k). We show how it is possible by means of the three stream-wise velocity component spectra to determine the three scalar functions in
ij
(k) by solving two uncoupled, ordinary linear differential equations of first and second order. The analytic form of the component spectra each has a set of three parameters: the variance and the integral length scale of the velocity component and a dimensionless parameter, which governs the curvature of the spectrum in the transition domain from the inertial subrange towards lower wave numbers. When the three sets of parameters are the same, the three spectra correspond to isotropic turbulence and they are all interrelated and related to the energy spectrum. We show how it is possible to obtain these spectral forms in the neutral surface layer and in the convective boundary layer from data reported in the literature. The spectral tensor is used to predict the lateral coherences for all three velocity components and these predictions are compared with coherences obtained in two experiments, one using three masts at a horizontally homogeneous site in Denmark and one employing two aircraft flying in formation over eastern Colorado. Comparison shows reasonable agreement although with considerable experimental scatter.The National Center for Atmospheric Research is sponsored by the National Science Foundation. 相似文献
9.
The chemical reactivity of NO and NO2 is so rapid that their fluxes and concentrations can be considerably modified from that expected for conserved variables in the atmospheric surface layer, even as low as a meter above the surface. Fitzjarrald and Lenschow (1983) have calculated flux and mean concentration profiles for NO, NO2 and O3 in the surface layer using numerical techniques. However, their solutions do not approach the photostationary state at large heights. Here we solve a simpler set of equations analytically (i.e. we assume a constant O3 concentration and neutral hydrodynamic stability), and are able to show how the flux profiles behave at large heights assuming that the concentrations approach their photostationary values. We find, for example, that at large heights the ratio of the flux of NO to that of NO2 is equal to the ratio of their concentrations. These results are relevant to estimating surface fluxes of NO and NO2, and are most applicable to nonurban environments where NO and NO2 concentrations are usually much less than O3 concentration.The National Center for Atmospheric Research is sponsored by the National Science Foundation. 相似文献
10.
Marie Lothon Fleur Couvreux Sylvie Donier Françoise Guichard Pierre Lacarrère Donald H. Lenschow Joël Noilhan Frédérique Saïd 《Boundary-Layer Meteorology》2007,124(3):425-447
During the Hydrological-Atmospheric Pilot Experiment (HAPEX)-Sahel, which took place in Niger in the transitional period between
the wet and dry seasons, two French aircraft probed the Sahelian boundary layer to measure sensible and latent heat fluxes.
The measurements over the Niamey area often revealed organised structures of a few km scale that were associated with both
thermals and dry intrusions. We study the impact of these coherent structures using a single day’s aircraft-measured fluxes
and a numerical simulation of that day with a mesoscale model. The numerical simulation at high horizontal resolution (250 m)
contains structures that evolve from streaks in the early morning to cells by noon. This simulation shows distribution, variance
and skewness similar to the observations. In particular, the numerical simulation shows dry intrusions that can penetrate
deeply into the atmospheric boundary layer (ABL), and even reach the surface in some cases, which is in accordance with the
observed highly negatively skewed water vapour fluctuations. Dry intrusions and thermals organised at a few km scale give
skewed flux statistics and can introduce large errors in measured fluxes. We use the numerical simulation to: (i) evaluate
the contribution of the organised structures to the total flux, and (ii) estimate the impact of the organised structures on
the systematic and random errors resulting from the 1D sampling of the aircraft as opposed to the 2D numerical simulation
estimate. We find a significant contribution by the organised structures to the total resolved fluxes. When rolls occur, and
for a leg length of about 30 times the ABL depth, the 1D sampled flux is shown to be sometimes 20% lower than the corresponding
2D flux when the 1D sampling direction is the same as the main axis of the rolls, whereas the systematic error is much lower
when the direction of the leg is transverse to the rolls. In the case of cells, an underestimate of around 10% can still be
observed with the 1D approach independent of direction, due to poor sampling of the energy-containing scales. 相似文献